You'd then have the confusion of two 'main' switches (visually anyway). Not sure if that would even be compliant - even though, yes the RCD will function in the same way. Best would be to put the left busbar straight off the main switch, and as you say, replace the MCBs with RCBOs.
The 'high integrity' came about with the trend of putting the freezer on it's own radial, and as long as it was labelled as being 'Freezer only' or similar, it didn't need to be RCD protected. The 'integrity' of not losing all your food!
That was my take on it anyway.
My comments have been flavoured due to my own problems. I had expected to find the problem reasonably fast, the replacement RCBOs are type A bidirectional double pole switching, but not the old ones, it said on the packet type B, but it seems they were curve B type AC single pole switching. So turning them off, does not allow testing neutral to earth with the insulation tester.
OK the isolator allowed testing neutral to earth for all circuits, but with the consumer unit in the flat, running up and down at my age was not what I want to do.
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